Laponite: Aging and Shear Rejuvenation of a Colloidal Glass

Daniel Bonn, Sorin Tanase, Bérengère Abou, Hajime Tanaka, and Jacques Meunier
Phys. Rev. Lett. 89, 015701 – Published 13 June 2002
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Abstract

We study the nonlinear rheological behavior and the microscopic particle dynamics for a colloidal glass, to see whether recently developed models for driven glassy systems can be applied to predict the rheology. Qualitatively, all the findings predicted by the models can be retrieved in our system. Notably, the viscosity decreases strongly with the shear rate. Since it is difficult to predict non-Newtonian viscosities of colloidal systems due to long-ranged hydrodynamic interactions, this shows the promise of this approach for predicting flow behavior. In addition, the measurements allow us to relate the microscopic diffusion dynamics to the macroscopic viscosity of the system.

  • Received 29 November 2001

DOI:https://doi.org/10.1103/PhysRevLett.89.015701

©2002 American Physical Society

Authors & Affiliations

Daniel Bonn1,*, Sorin Tanase1, Bérengère Abou1,†, Hajime Tanaka2, and Jacques Meunier1

  • 1Laboratoire de Physique Statistique, Ecole Normale Supérieure, 24, rue Lhomond, 75005 Paris, France
  • 2Institute of Industrial Science, University of Tokyo, Minato-ku, Tokyo 106, Japan

  • *Electronic address: bonn@lps.ens.fr
  • Present address: LBHP, Universite Paris 7, LBHP, 2, place Jussieu, F-75251 Paris Cedex 05, France.

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Vol. 89, Iss. 1 — 1 July 2002

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