Coherence signatures and density-dependent interaction in a dynamical exciton-polariton condensate

A. Rahimi-Iman, A. V. Chernenko, J. Fischer, S. Brodbeck, M. Amthor, C. Schneider, A. Forchel, S. Höfling, S. Reitzenstein, and M. Kamp
Phys. Rev. B 86, 155308 – Published 11 October 2012

Abstract

We report on pump-power-dependent emission features of a nonthermalized and interacting dynamical condensate of exciton polaritons. The system based on a planar AlAs/AlGaAs microcavity sample with twelve GaAs quantum wells in the active region is investigated comprehensively by measuring the energy-momentum dispersion characteristics, the spatial coherence, and the photon statistics under resonant, fs-pulsed optical excitation at high momentum. We observe a significant polariton-population-dependent modification of the emission signatures above the quantum degeneracy. The nonequilibrium polariton condensate is confirmed by its polaritonic energy-momentum dispersion as well as excitation-power-dependent coherence properties and its photon statistics, being different from that of an ideal coherent state. The polaritonic condensate is characterized by a spatial coherence length of up to 4 μm and a super-Poissonian photon statistic of the emitted light well above threshold. Results obtained in second-order photon autocorrelation measurements in momentum-space resolved spectroscopy indicate polariton repulsive interaction throughout the condensate and a spatial coherence length being shorter than the condensate extension of 20–30 μm.

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  • Received 19 May 2012

DOI:https://doi.org/10.1103/PhysRevB.86.155308

©2012 American Physical Society

Authors & Affiliations

A. Rahimi-Iman1,*, A. V. Chernenko2, J. Fischer1, S. Brodbeck1, M. Amthor1, C. Schneider1, A. Forchel1, S. Höfling1, S. Reitzenstein1,†, and M. Kamp1

  • 1Technische Physik, Physikalisches Institut and Wilhelm Conrad Röntgen Research Center for Complex Material Systems, Universität Würzburg, Am Hubland, D-97074 Würzburg, Germany
  • 2Institute of Solid State Physics, Russian Academy of Sciences, Chernogolovka, 142432 Russia

  • *arash.rahimi-iman@physik.uni-wuerzburg.de
  • Present address: Institut für Festkörperphysik, Technische Universität Berlin, Hardenbergstrasse 36, D-10623 Berlin, Germany.

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Vol. 86, Iss. 15 — 15 October 2012

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