Proximate Quantum Spin Liquid on Designer Lattice

Liu, Xiaoran; Singh, Sobhit; Drouin-Touchette, Victor; Asaba, Tomoya; Brewer, Jess; Zhang, Qinghua; Cao, Yanwei; Pal, Banabir; Middey, Srimanta; Kumar, P. Anil; Kareev, Mikhail; Gu, Lin; Sarma, D. D.; Shafer, Padraic; Arenholz, Elke; Freeland, John W.; Li, Lu; Vanderbilt, David; Chakhalian, Jak

doi:10.1021/acs.nanolett.0c04498

Title: Proximate Quantum Spin Liquid on Designer Lattice

Journal Article · Mon Feb 22 00:00:00 EST 2021 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.0c04498· OSTI ID:1797949

^[1]; Singh, Sobhit ^[1]; Drouin-Touchette, Victor ^[1]; Asaba, Tomoya ^[2]; Brewer, Jess ^[3]; Zhang, Qinghua ^[4]; Cao, Yanwei ^[5]; Pal, Banabir ^[6];

^[7];

^[7]; Kareev, Mikhail ^[1];

^[4]; Sarma, D. D. ^[7];

^[8]; Arenholz, Elke ^[8]; Freeland, John W. ^[9]; Li, Lu ^[2]; Vanderbilt, David ^[1]; Chakhalian, Jak ^[1]

Rutgers Univ., Piscataway, NJ (United States)
Univ. of Michigan, Ann Arbor, MI (United States)
TRIUMF, Vancouver, BC (Canada); Univ. of British Columbia, Vancouver, BC (Canada)
Chinese Academy of Sciences (CAS), Beijing (China)
Chinese Academy of Sciences, Zhejiang (China)
Rutgers Univ., Piscataway, NJ (United States); Indian Inst. of Science, Bengaluru (India)
Indian Inst. of Science, Bengaluru (India)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Complementary to bulk synthesis, here we propose a designer lattice with extremely high magnetic frustration and demonstrate the possible realization of a quantum spin liquid state from both experiments and theoretical calculations. In an ultrathin (111) CoCr₂O₄ slice composed of three triangular and one kagome cation planes, the absence of a spin ordering or freezing transition is demonstrated down to 0.03 K, in the presence of strong antiferromagnetic correlations in the energy scale of 30 K between Co and Cr sublattices, leading to the frustration factor of similar to 1000. Persisting spin fluctuations are observed at low temperatures via low-energy muon spin relaxation. Our calculations further demonstrate the emergence of highly degenerate magnetic ground states at the 0 K limit, due to the competition among multiply altered exchange interactions. Furthermore, these results collectively indicate the realization of a proximate quantum spin liquid state on the synthetic lattice.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; Gordon and Betty Moore Foundation

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1797949

Journal Information:: Nano Letters, Vol. 21, Issue 5; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Proximate Quantum Spin Liquid on Designer Lattice

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