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Recent advances in perovskite/organic integrated solar cells

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Abstract

The integrated perovskite/organic solar cell (IPOSC) is widely concerned as an effective approach to broaden the spectrum of perovskite solar cell (PerSC) by utilizing near-infrared light of lower bandgap organic semiconductor. Compared to tandem solar cells, the IPOSCs eliminate the preparation of the intermediate layer and simplify the manufacturing process, but retain the advantages of wide light harvesting. Meanwhile, the IPOSCs can maintain the open-circuit voltage as high as PerSCs. This review summarizes the recent developments of perovskite materials and low-bandgap organic conjugated materials applied in solar cells. Then, the working mechanism of IPOSCs and the recent developments of IPOSCs based on low-bandgap donor and acceptor materials are highlighted. Besides, the study of charge dynamic in IPOSC is summarized. Finally, the potential of IPOSCs and approach to improve device performance are also envisaged.

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Fig. 1

Reproduced with permission from Ref. [10]. Copyright 2020 WILEY–VCH. c Normalized absorption spectrum of perovskite layer and BHJ layer in IPOSCs. Reproduced with permission from Ref. [7]. Copyright 2019 WILEY–VCH

Fig. 2

Reproduced with permission from Ref. [16]. Copyright 2014 Macmillan Publishers Limited. b UV–Vis spectra for APbI3 perovskites formed, where Position A is either cesium (Cs), methylammonium (MA) or formamidinium (FA). Reproduced with permission from Ref. [20]. Copyright 2014 The Royal Society of Chemistry

Fig. 3

Reproduced with permission from Ref. [25]. Copyright 2014 American Chemical Society. c Absorption spectra and d normalized PL spectra of (FASnI3)1-x(MAPbI3)x perovskites with x = 0, 0.2, 0.4, 0.6, 0.9, and 1.0. Reproduced with permission from Ref. [24]. Copyright 2016 American Chemical Society

Fig. 4
Fig. 5

Reproduced with permission from Ref. [5]. Copyright 2015 The Royal Society of Chemistry. c J-V and d EQE curves for PDPP3T:PCBM OSCs, PerSCs and CH3NH3PbI3/PDPP3T:PC61BM IPOSCs. Reproduced with permission from Ref. [46]. Copyright 2015 Elsevier. e J-V, f EQE curves and integrated Jsc for perovskite/PCBM PerSCs and perovskite/PDPP3T:PC61BM IPOSCs. Reproduced with permission from Ref. [47]. Copyright 2015 Science China Press and Springer-Verlag Berlin Heidelberg. g J-V curves, h EQE and absorption spectra for PerSCs with PBDTT-SeDPP HTL and IPOSCs with PBDTT-SeDPP:PC71BM. Reproduced with permission from Ref. [6]. Copyright 2015 American Chemical Society. i J-V and j IPCE curves of IPOSCs containing M3:PC70BM or M4:PC70BM BHJ HTLs. Reproduced with permission from Ref. [48]. Copyright 2016 American Chemical Society. k J-V and l EQE curves of optimized PerSCs (PC61BM) and IPOSCs incorporating CB, CB:DPE, and CB:DPE:N2200 processed BHJ films. Reproduced with permission from Ref. [49]. Copyright 2016 WILEY–VCH; m J-V and n EQE curves for CH3NH3PbI3/PCBM PerSCs and CH3NH3PbI3/TT:PCBM:N2200 IPOSCs. Reproduced with permission from Ref. [50]. Copyright 2020 WILEY–VCH. o J-V and p EQE curves of optimized IPOSCs with 110-nm-thick DPPZnP-TSEH:PC61BM film and optimized PerSC with Spiro-OMeTAD as HTL. Reproduced with permission from Ref. [50]. Copyright 2020 WILEY–VCH

Fig. 6

Reproduced with permission from Ref. [52]. Copyright 2018 The Royal Society of Chemistry. c J-V and d EQE curves for CH3NH3PbI3/PBDB-T:IEICO IPOSCs with different weight ratios of PBDB-T and IEICO. Reproduced with permission from Ref. [53]. Copyright 2019 The Royal Society of Chemistry. e J-V, f EQE curves (inset being J-V curves obtained in dark environment of OSCs (pink), PerSCs (red) and IPOSCs (blue)) and integrated Jsc for PBDTTT-E-T:IEICO OSCs (pink), CsPbI2Br/spiro-OMeTAD PerSCs (red) and CsPbI2/PBDTTT-E-T:IEICO IPOSCs (blue). Reproduced with permission from Ref. [54]. Copyright 2019 American Chemical Society; g J-V curves of CsPbBr3/J61:ITIC and Cs0.91Rb0.09PbBr3/J61:ITIC IPOSCs, h IPCE of CsPbBr3 PerSCs and CsPbBr3/J61:ITIC IPOSCs. Reproduced with permission from Ref. [55]. Copyright 2019 Elsevier. i J-V and j EQE spectra of (FAPbI3)0.85(MAPbBr3)0.15 PerSCs using a bare PCBM ETL and IPOSCs with optimized T-PCE13 ETL. Reproduced with permission from Ref. [56]. Copyright 2019 WILEY–VCH. k J-V curves of device based on different active layers and l EQE curves and calculated JSC curves of perovskite/PTB7-Th (black), perovskite/PTB7-Th:PCBM (blue), perovskite/PTB7-Th:F8IC (red), and PTB7-Th:F8IC (green). Reproduced with permission from Ref. [57]. Copyright 2020 WILEY–VCH. m J-V and n EQE curves for perovskite/PCBM PerSCs and perovskite/Y6:PCBM:S1 IPOSCs. Reproduced with permission from Ref. [13]. Copyright 2019 American Chemical Society. o J-V and p EQE curves for perovskite/PCBM PerSCs and perovskite/Y6:PCBM:S2 IPOSCs. Reproduced with permission from Ref. [58]. Copyright 2019 Science China Press

Fig. 7

Reproduced with permission from Ref. [46]. Copyright 2015 Elsevier

Fig. 8

Reproduced with permission from Ref. [12]. Copyright 2017 American Chemical Society

Fig. 9

Reproduced with permission from Ref. [12]. Copyright 2017 American Chemical Society

Fig. 10

Reproduced with permission from Ref. [54]. Copyright 2019 American Chemical Society. c TAS of films at pump-probe delay of 2 ps and d kinetic traces of perovskite with and without BHJ and perovskite/spiro-OMeTAD at wavelength of 750 nm; e magnified view of c; f kinetic traces of ground state bleaching below bandgap of perovskite. Reproduced with permission from Ref. [51]. Copyright 2017 WILEY–VCH. g TAS kinetics of perovskite, BHJ, perovskite/BHJ layers with excitation at 550 nm, where TAS signal of TT are probed at a laser wavelength of 840 nm. Reproduced with permission from Ref. [50]. Copyright 2020 WILEY–VCH. (OD representing optical density; ΔA and ΔOD representing change in optical density; ΔmOD = ΔOD/1000)

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Acknowledgements

This work was financially supported by the National Key Research and Development Program of China (No. 2016YFA0202401), the National Natural Science Foundation of China (Nos. 51873007, 51961165102 and 21835006), the Fundamental Research Funds for the Central Universities in China (No. 2019MS025), the State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources (No. LAPS20003) and the Outstanding Talent Research Fund of Zhengzhou University (No. 32340035).

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  1. Qiang Guo and Chen-Yun Wang have contributed equally to this work.

Authors and Affiliations

  1. Henan Institute of Advanced Technology, Zhengzhou University, Zhengzhou, 450002, China

    Qiang Guo

  2. State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources, North China Electric Power University, Beijing, 102206, China

    Chen-Yun Wang & Jian-Xi Yao

  3. Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100090, China

    Zhan-Ao Tan

  4. NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia

    Tasawar Hayat & Ahmed Alsaedi

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Guo, Q., Wang, CY., Hayat, T. et al. Recent advances in perovskite/organic integrated solar cells. Rare Met. 40, 2763–2777 (2021). https://doi.org/10.1007/s12598-020-01703-y

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