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Mesoporous Hierarchically Hollow Flower-Like CoAl-LDH@N,S-doped Graphene@Pd Nanoarchitectures for Heck Couplings

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Abstract

A smart strategy for the synthesis of hierarchical CoAl-LDH hollow spheres assembled with nitrogen and sulfur co-doped graphene for high holding of palladium nanoparticles (CoAl-LDH@N,S-G@Pd) is reported. This architecture exhibited excellent activity in Heck reactions with TOF as high as 1633 h−1 due to a strong metal–support interaction, good electron transfers and high surface area.

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Acknowledgements

The financial support from the research council of Alzahra University and the University of Tehran are gratefully acknowledged. The publication was prepared with support from RUDN University Program 5-100.

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Authors and Affiliations

  1. Department of Chemistry, Faculty of Science, University of Alzahra, Tehran, Iran

    Sahar Rohani & Ghodsi Mohammadi Ziarani

  2. School of Chemistry, College of Science, University of Tehran, Tehran, Iran

    Alireza Badiei & Abolfazl Ziarati

  3. Departamento de Quimica Organica, Universidad de Cordoba, Campus de Rabanales, Edificio Marie Curie, 14014, Córdoba, Spain

    Rafael Luque

  4. Peoples Friendship University of Russia (RUDN University), 6 Miklukho Maklaya str, Moscow, Russia, 117198

    Rafael Luque

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  1. Sahar Rohani
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  2. Ghodsi Mohammadi Ziarani
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  3. Alireza Badiei
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  4. Abolfazl Ziarati
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  5. Rafael Luque
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Correspondence to Ghodsi Mohammadi Ziarani.

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Rohani, S., Mohammadi Ziarani, G., Badiei, A. et al. Mesoporous Hierarchically Hollow Flower-Like CoAl-LDH@N,S-doped Graphene@Pd Nanoarchitectures for Heck Couplings. Catal Lett 149, 2984–2993 (2019). https://doi.org/10.1007/s10562-019-02880-x

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