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Pt–Ru electrocatalysts for fuel cells: a representative review

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Abstract

Three periods of Pt–Ru research are considered step-by-step: the initial period after discovery (1963–1970); observation and classification of basic tendencies (like the effects of composition, segregation, structural features on the activity; up to 1990); nanostructural studies and molecular level consideration of electrocatalytic phenomena in combination with advanced applied studies of materials, mechanistic, and applied aspects (after 1990). The main idea of this review is to balance various aspects of Pt–Ru electrochemistry related to material science and electrocatalysis as well as to remember the early basic results being of importance for future understanding of Pt–Ru functional properties.

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Notes

  1. The basis of this review is the lecture “Ru-containing catalysts—a very long story” presented at 55th ISE Meeting in Tessaloniki, September 2004.

  2. Publication of monograph [162] devoted to ruthenium chemistry should be mentioned.

  3. State-of-the art in electrocatalysis at the beginning of the third period was vividly presented by Pletcher [163].

  4. Abbreviations: dba—dibenzylidene acetone; COD—1,5-cyclooctadiene; COT—1,3,5-cyclooctatriene.

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Acknowledgements

I am grateful to Prof. G.A. Tsirlina for her active stimulating criticism in the course of review preparation. I would like to acknowledge the referees whose valuable remarks were extremely helpful. Pt–Ru research is supported by RFBR, project 05-03-32592a.

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  1. Department of Electrochemistry, Moscow State University, Leninskie Gory 1-str.3, Moscow, 119992, Russia

    Oleg A. Petrii

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Correspondence to Oleg A. Petrii.

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Dedicated to Professor Teresa Iwasita, as a token of her remarkable contribution to electrocatalysis.

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Petrii, O.A. Pt–Ru electrocatalysts for fuel cells: a representative review. J Solid State Electrochem 12, 609–642 (2008). https://doi.org/10.1007/s10008-007-0500-4

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