Abstract
Crystalline polymers may be affected by various kinds and amounts of structural disorder. Lackof order in polymer crystals may arise from the presence of defects in the chemical constitution,configuration and conformation and defects in the mode of packing of chains inside the crystals. Polymericmaterials characterized by long range order in the parallel arrangement of chain axes and a largeamount of structural disorder may be considered as solid mesophases. The different kinds and amountof disorder present in the solid mesophases of semicrystalline polymers and the possible types ofsolid mesophases are discussed in terms of idealized limit models of disorder. These models implymaintenance of long-range positional order, at least along one dimension, of structural features whichare not necessarily point centered. Structural features, which are not point centered, are for instancechain axes, the center of mass of special groups of atoms or bundles of chains and so on. Structuralaspects emerging from the X-ray diffraction analysis of several solid mesophases discussed so farin the literature are reviewed, in the light of the present analysis.
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Auriemma, F., De Rosa, C., Corradini, P. (2005). Solid Mesophases in Semicrystalline Polymers: Structural Analysis by DiffractionTechniques. In: Allegra, G. (eds) Interphases and Mesophases in Polymer Crystallization II. Advances in Polymer Science, vol 181. Springer, Berlin, Heidelberg. https://doi.org/10.1007/b107169
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